Beyond Fossil Fuel-Driven Nitrogen Transformations

Jingguang G. Chen; Richard M. Crooks; Lance C. Seefeldt; Kara L. Bren; R. Morris Bullock; Marcetta Y. Darensbourg; Patrick L. Holland; Brian Hoffman; Michael J. Janik; Anne K. Jones; Mercouri G. Kanatzidis; Paul King; Kyle M. Lancaster; Sergei V. Lymar; Peter Pfromm; William F. Schneider; Richard R. Schrock

doi:10.1126/science.aar6611

Beyond Fossil Fuel-Driven Nitrogen Transformations

Jingguang G. Chen
, Richard M. Crooks
, Lance C. Seefeldt
, Kara L. Bren
, R. Morris Bullock
, Marcetta Y. Darensbourg
, Patrick L. Holland
, Brian Hoffman
, Michael J. Janik
, Anne K. Jones
, Mercouri G. Kanatzidis
, Paul King
, Kyle M. Lancaster
, Sergei V. Lymar
, Peter Pfromm
, William F. Schneider
, Richard R. Schrock

Biosciences Center

Columbia University
Brookhaven National Laboratory
University of Texas at Austin
Utah State University
University of Rochester
Pacific Northwest National Laboratory
Texas A&M University
Yale University
Northwestern University
Pennsylvania State University
Arizona State University
Cornell University
Washington State University Pullman
University of Notre Dame
Massachusetts Institute of Technology

Research output: Contribution to journal › Article › peer-review

1950 Scopus Citations

Abstract

Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review.

Original language	American English
Article number	eaar6611
Number of pages	7
Journal	Science
Volume	360
Issue number	6391
DOIs	https://doi.org/10.1126/science.aar6611 https://doi.org/10.1126/science.aar6611
State	Published - 25 May 2018

Bibliographical note

Publisher Copyright:
2017 © The Authors.

NLR Publication Number

NREL/JA-2700-70628

Keywords

chemistry
fossil fuels
nitrogen

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Chen, J. G., Crooks, R. M., Seefeldt, L. C., Bren, K. L., Morris Bullock, R., Darensbourg, M. Y., Holland, P. L., Hoffman, B., Janik, M. J., Jones, A. K., Kanatzidis, M. G., King, P., Lancaster, K. M., Lymar, S. V., Pfromm, P., Schneider, W. F., & Schrock, R. R. (2018). Beyond Fossil Fuel-Driven Nitrogen Transformations. Science, 360(6391), Article eaar6611. https://doi.org/10.1126/science.aar6611, https://doi.org/10.1126/science.aar6611

@article{69745cd102794e3780fe39e659d178d9,

title = "Beyond Fossil Fuel-Driven Nitrogen Transformations",

abstract = "Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review.",

keywords = "chemistry, fossil fuels, nitrogen",

author = "Chen, \{Jingguang G.\} and Crooks, \{Richard M.\} and Seefeldt, \{Lance C.\} and Bren, \{Kara L.\} and \{Morris Bullock\}, R. and Darensbourg, \{Marcetta Y.\} and Holland, \{Patrick L.\} and Brian Hoffman and Janik, \{Michael J.\} and Jones, \{Anne K.\} and Kanatzidis, \{Mercouri G.\} and Paul King and Lancaster, \{Kyle M.\} and Lymar, \{Sergei V.\} and Peter Pfromm and Schneider, \{William F.\} and Schrock, \{Richard R.\}",

note = "Publisher Copyright: 2017 {\textcopyright} The Authors.",

year = "2018",

month = may,

day = "25",

doi = "10.1126/science.aar6611",

language = "American English",

volume = "360",

journal = "Science",

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Chen, JG, Crooks, RM, Seefeldt, LC, Bren, KL, Morris Bullock, R, Darensbourg, MY, Holland, PL, Hoffman, B, Janik, MJ, Jones, AK, Kanatzidis, MG, King, P, Lancaster, KM, Lymar, SV, Pfromm, P, Schneider, WF & Schrock, RR 2018, 'Beyond Fossil Fuel-Driven Nitrogen Transformations', Science, vol. 360, no. 6391, eaar6611. https://doi.org/10.1126/science.aar6611, https://doi.org/10.1126/science.aar6611

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T1 - Beyond Fossil Fuel-Driven Nitrogen Transformations

AU - Chen, Jingguang G.

AU - Crooks, Richard M.

AU - Seefeldt, Lance C.

AU - Bren, Kara L.

AU - Morris Bullock, R.

AU - Darensbourg, Marcetta Y.

AU - Holland, Patrick L.

AU - Hoffman, Brian

AU - Janik, Michael J.

AU - Jones, Anne K.

AU - Kanatzidis, Mercouri G.

AU - King, Paul

AU - Lancaster, Kyle M.

AU - Lymar, Sergei V.

AU - Pfromm, Peter

AU - Schneider, William F.

AU - Schrock, Richard R.

PY - 2018/5/25

Y1 - 2018/5/25

N2 - Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review.

AB - Nitrogen is fundamental to all of life and many industrial processes. The interchange of nitrogen oxidation states in the industrial production of ammonia, nitric acid, and other commodity chemicals is largely powered by fossil fuels. A key goal of contemporary research in the field of nitrogen chemistry is to minimize the use of fossil fuels by developing more efficient heterogeneous, homogeneous, photo-, and electrocatalytic processes or by adapting the enzymatic processes underlying the natural nitrogen cycle. These approaches, as well as the challenges involved, are discussed in this Review.

KW - chemistry

KW - fossil fuels

KW - nitrogen

UR - https://www.scopus.com/pages/publications/85047437217

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DO - 10.1126/science.aar6611

M3 - Article

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AN - SCOPUS:85047437217

SN - 0036-8075

VL - 360

JO - Science

JF - Science

IS - 6391

M1 - eaar6611

ER -

Beyond Fossil Fuel-Driven Nitrogen Transformations

Abstract

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Keywords

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